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Decay Kraus weights and photon overlap

PDF p. 7: Paragraph before Fig. 5 and upper right paragraph

Statement

Assume the four-level model with fixed real ω0,Δ, fixed γ>0, and t>0. Let K2,K3 be the model's decay Kraus operators, p=1−e−γt, and χ=γ(eiΔt−e−γt)/[(γ+iΔ)p] as its conditional decay coherence. Define the weight of an operator as wj=Tr⁡(Kj†Kj). Then w2,3=p(1±∣χ∣), with the upper sign for K2. The fraction of the sum of the two decay weights carried by K3 is (1−∣χ∣)/2. For fixed γ,Δ, as t↓0 this fraction is Δ2t2/48+O(t3), and as t→∞ it tends to [1−γ/γ2+Δ2]/2.

The two operators are respectively the sum and difference of the two decay-path operators after a relative phase adjustment, as represented by the signs in Fig. 5. In an environmental realization in which the normalized emitted-photon path states have overlap χ in the convention below, their overlap modulus is ∣χ∣. The reduced-system model alone does not identify a unique measured photon state. At t=0 or γ=0 both decay weights vanish; their normalized fraction and the conditional coherence are then undefined.

Facts & Assumptions

[F1]

The model has orthonormal basis ∣0⟩,…,∣3⟩, with decay paths F0=∣2⟩⟨0∣ and F1=∣3⟩⟨1∣. Adjoints, outer products and the coordinate inner product use the finite operator conventions. Four-level spontaneous-decay model Finite operator and ket conventions

[F2]

For γt>0, the decay probability and coherence are p=1−e−γt and χ=γ(eiΔt−e−γt)/[(γ+iΔ)p]. Conditional decoded state and decay coherence

[F3]

The two decay Kraus operators are those in Exact four-level Kraus operators. With Ω=γ+iΔ, that result supplies f±=γ∣eΩt−1∣/∣Ω∣±(eγt−1) and a unit-modulus phase u, with K2=e−γt/2f+/2(uF0+F1) and K3=e−γt/2−f−/2(−uF0+F1). For positive γ,t, its derivation gives the one-jump coefficients p and pχ and u=χ/∣χ∣. Its square roots are real and nonnegative, and both operators are zero at zero decay probability.

[F4]

For a two-path branch with coefficient matrix p(1χχ‾1), p>0 and ∣χ∣≤1, the orthogonal Kraus weights are p(1±∣χ∣) and the smaller fraction is (1−∣χ∣)/2. Its eigenoperators are the phase-adjusted sum and difference of the two paths. Two-path coherence Gram spectrum and Kraus weights

[F5]

For a finite list of vectors in an inner product space, its Gram matrix has entries Gjk=⟨vj,vk⟩. Here the coordinate inner product is linear in its first argument. The Gram matrix G(v₀,…,vᵣ₋₁)=(⟨ vᵢ,vⱼ⟩)_i,j<r and Gram determinant, with empty value 1 Finite operator and ket conventions

[F6]

Scalar exponential expansions and quotient expansions with nonzero constant denominator have controlled remainders at fixed parameters. Finite exponential and smooth quotient remainder control

[F7]

The trace of a square matrix is the sum of its diagonal entries. We use Tr⁡ for this matrix trace in the fixed model basis. The trace tr(A) as the sum of the diagonal entries

Proof

Given: The model, positive rate and time, and the definitions in the Statement.

Goal: Derive the weights, fraction, limits and the stated conditional overlap interpretation.

1.1givenF1F2F3F4algebra

Put r=∣χ∣ and Ω=γ+iΔ. Here 0<p<1 and Ω≠0. The formula in [F2] gives pr=γe−γt∣eΩt−1∣/∣Ω∣, hence e−γtf+=p(1+r) and −e−γtf−=p(1−r). The real square root of −f−/2 supplied by [F3] implies f−≤0, so r≤1. The two-path branch on the code therefore satisfies the hypotheses of [F4]; both path maps annihilate the orthogonal decay space. This argument invokes the already established Kraus representation, independently of the weight identities proved below.

2.1F1F3F4F7step 1.1algebra

By [F1], F0†F1=F1†F0=0, F0†F0=∣0⟩⟨0∣ and F1†F1=∣1⟩⟨1∣. Write Π01=∣0⟩⟨0∣+∣1⟩⟨1∣. Since ∣u∣=1, [F3] and step 1.1 give K2†K2=p(1+r)Π01/2 and K3†K3=p(1−r)Π01/2. In the four-level basis Π01 has diagonal (1,1,0,0), so [F7] gives w2,3=p(1±r). Equivalently, summing the diagonal entries of Kj†Kj gives the sum of the squared moduli of all entries of Kj, its squared Hilbert–Schmidt norm. The two extra input columns outside the code are zero. The weight sum is 2p, and the K3 fraction is (1−r)/2. The displayed operators are the phase-adjusted sum and difference directions of [F4], up to the overall sign of the minus operator; this explains the signs in Fig. 5 without asserting a unique measured trajectory.

3.1givenF2F6step 2.1algebra

Cancel the common factor t in the numerator and denominator of χ. By [F6], expansion at fixed γ,Δ gives χ=1+iΔt/2+(−Δ2/6+iγΔ/12)t2+O(t3). Consequently ∣χ∣2=1−Δ2t2/12+O(t3) and ∣χ∣=1−Δ2t2/24+O(t3); the last equality follows from ∣χ∣−1=(∣χ∣2−1)/(∣χ∣+1). Substitution into step 2.1 gives Δ2t2/48+O(t3).

3.2givenF2F3step 2.1algebra

Since e−γt→0 for fixed γ>0, [F2] gives ∣χ∣=γ∣eiΔt−e−γt∣/[γ2+Δ2(1−e−γt)]→γ/γ2+Δ2. Step 2.1 gives the asserted limiting fraction. At t=0 or γ=0, [F3] gives K2=K3=0, and [F2] supplies no conditional decay coherence at zero probability.

4.1givenF1F5step 1.1step 2.1step 3.1step 3.2algebra∎

For an explicit normalized overlap model, take the finite coordinate space C2 with the inner product of [F1], and put v0=(χ,1−r2) and v1=(1,0). Step 1.1 makes the square root real and nonnegative. Coordinate calculation gives ⟨v0,v0⟩=∣χ∣2+1−r2=1, ⟨v1,v1⟩=1 and ⟨v0,v1⟩=χ. Thus [F5] identifies their Gram matrix as (1χχ‾1), the same coefficient matrix as the normalized two-path branch. If a physical environmental realization identifies this normalized path-state Gram matrix with that of its emitted photons, their overlap modulus is ∣χ∣. That identification remains an additional physical interpretation, not a consequence of the reduced channel alone. Together with steps 2.1, 3.1 and 3.2 this proves the conditional assertions.

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