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Three spherical emission channels

PDF p. 13: Eq. (S3.17) and following paragraph

Statement

Assume the Axiom of Choice, Countable Choice and Dependent Choice. Take the finite-dimensional static system, three Hermitian Cartesian coupling operators Xx,Xy,Xz, stationary Gaussian bath, preparation, weak-Markov regime, Fourier identities and kernel regularity required by the static ULE result. Also take the regulated isotropic thermal photon model and its limit under the hypotheses of the isotropic-bath result. Require that its nonnegative scalar spectral representative J agrees pointwise at every required transition frequency with the ordinary spectral density in the static ULE result, and that the latter's remaining hypotheses hold. In particular γ>0 is the coupling scale in that ULE convention, and all square roots below are nonnegative.

Work in the inherited units ℏ=1, so the energies in HS are angular frequencies. For a finite family L=(La) on the system space define its dissipator on every system matrix ρ by DL(ρ)=∑a(LaρLa†−12La†Laρ−12ρLa†La), where † denotes conjugate transpose. This is the dissipative part of the finite GKSL generator. To compare units with its supplier, fix a time unit T>0 seconds and an action unit A>0 joule-seconds: the numerical matrices here correspond to La/T, physical Planck constant A, and physical Hamiltonian (A/T)HS there. Multiplication of that physical generator by T gives the convention used here. The channel rotation below leaves the Hamiltonian part fixed.

Choose an orthonormal energy eigenbasis HS∣n⟩=En∣n⟩ and put ωmn=En−Em. Define X+1=−(Xx+iXy)/2, X−1=(Xx−iXy)/2 and X0=Xz. A valid unitary choice of the three ULE jump operators is

Lq=2πγ∑m,nJ(ωmn)⟨m∣Xq∣n⟩∣m⟩⟨n∣,q∈{−1,0,+1}.

The article denotes this channel label by δ in its main text. For the angular-momentum interpretation, additionally suppose the system basis consists of magnetic eigenvectors and the Xq form a rank-one spherical tensor. Specify the emission process by the following local physical assumptions. Let R be a set of remainder-field records and P a set of single-photon records, with real-valued maps r:R→R and s:P→R assigning angular-momentum projections on the chosen axis in units of ℏ. The initial field record is a∈R, with projection r(a)=0; the final field record is (b,p)∈R×P, consisting of the remainder b and exactly one emitted photon p, with projection r(b)+s(p). Assume the remainder projection is unchanged, r(b)=r(a), and the transition conserves the sum of system and field projections. These record types and additive assignments are assumptions for this interpretation; they assert no general factorization of a thermal field. If the system matrix element for that transition is nonzero, the emitted photon's projection is s(p)=−q. This assertion concerns the projection and the stated emission process; the formula alone does not exclude absorption at nonzero temperature.

Facts & Assumptions

[F1]

Under its stated system, bath, preparation, weak-Markov and regularity hypotheses, the static ULE result gives Li=2πγ∑m,n,jgij(ωmn)⟨m∣Xj∣n⟩∣m⟩⟨n∣, with g=[J/(2π)]1/2. Static ULE formulas and principal-value kernel Stationary correlation spectra and ULE kernel regularity

[F2]

Under the stated isotropic photon-model hypotheses, the spectral matrix has a scalar nonnegative representative and its positive jump correlator is the corresponding scalar square root times the identity. The isotropic result requires the three stated choice assumptions. Off-diagonal correlators vanish in an isotropic photon bath The Axiom of Choice The Axiom of Countable Choice (AC_ω) The axiom of dependent choice: a relation in which every element is related to something admits an ℕ-indexed chain

[F3]

The displayed spherical components are obtained from the Cartesian components by a unitary coefficient matrix U; ωmn is source energy minus destination energy. Spherical vector components and transition-frequency convention

[F4]

A rank-one spherical tensor satisfies [Jz,Xq]=qXq. Equivalently, its matrix elements between magnetic eigenvectors vanish unless the final system magnetic label equals the initial label plus q. Finite spin blocks, spherical tensors and Clebsch–Gordan phases Wigner–Eckart with explicit magnetic-label contract

[F5]

The finite GKSL definition supplies the dissipator DL displayed in the Statement; its supplier has domain mathematics. The finite system dimension and the three finite jump matrices meet its algebraic hypotheses, and the positive units T,A specified above convert its physical units to the inherited ℏ=1 convention. No microscopic approximation is inferred from that definition. Finite GKSL generators and units

[A1]

Assume the choice, matching, regularity and physical hypotheses in the Statement, including the locally specified field-record, additivity, unchanged-remainder and conservation hypotheses only for the final interpretation.

Proof

Given: The system, bath, spectral matching and choice hypotheses in the Statement; for the final assertion, also the stated tensor and local field-record assumptions, including additivity, unchanged remainder projection and conservation.

Goal: Derive the three displayed jump operators and the conditional photon-projection label.

1.1givenA1F1F2algebra

At each required transition frequency, [F2] and the pointwise matching assumption give gij(ωmn)=δijJ(ωmn)/(2π). Substitution into [F1] gives Li=2πγ∑m,nJ(ωmn)⟨m∣Xi∣n⟩∣m⟩⟨n∣ for the Cartesian labels. The coefficient is real and nonnegative by the specified representative.

2.1F3F5step 1.1algebra

Let Lq=∑iUqiLi, with i=x,y,z. By [F3], ∑qUqiUqj‾=δij, so expansion of the finite sums gives ∑qLqρLq†=∑iLiρLi† and ∑qLq†Lq=∑iLi†Li. Substituting these identities into the definition in [F5] gives D(Lq)(ρ)=D(Li)(ρ) for every system matrix ρ; the unchanged Hamiltonian part therefore gives the same ULE generator. Linearity of matrix elements and [F3] turn the Cartesian expression from step 1.1 into the displayed formula with Xq=∑iUqiXi. Thus it is a valid choice of the three jump operators.

3.1givenA1F4algebra∎

Write μin and μout for the initial and final system magnetic labels. For a nonzero matrix element, [F4] gives μout−μin=q. Under the local assumptions in [A1], conservation is μin+r(a)=μout+r(b)+s(p). Since r(b)=r(a), subtraction yields s(p)=μin−μout=−q. The additive field assignment identifies this scalar as the emitted photon's projection. The remainder may contain other excitations, but its projection must be unchanged; conservation alone would only give s(p)=−q+r(a)−r(b). This proves the stated conditional interpretation.

Source notes

The article uses the same symbol for the scalar bath spectrum in its spherical formula and describes γ as an effective decay scale. Here the normalization is fixed by the completed ULE and isotropic-bath interfaces, with pointwise matching explicitly required. The article's −q description is retained as a projection balance under the stated tensor, conservation, additive field-record and unchanged-remainder assumptions. The field-record model is a local physical assumption, not an imported fact from the article. The source passage is attribution, not a premise for that balance.

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