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Commutator and spontaneous-plus-stimulated emission contribution

PDF p. 12: Eqs. (S3.9)–(S3.11)

Statement

Assume the Axiom of Choice, Countable Choice and Dependent Choice, and adopt the finite-mode thermal-bath, regularized photon-mode and real-polarization dipole-coupling postulates. Let j=1,…,m, m≥1, index independent bosonic modes of frequencies ωj>0, and let β>0 and γ>0. Write aj,aj† for the annihilation and creation operators, ∣n⟩ for the occupation basis, HB=∑jωjaj†aj, Z=∏j(1−e−βωj)−1, and ρB=Z−1e−βHB. Put Nj=(eβωj−1)−1 and Pαj=e^α⋅ϵj, where e^α is a Cartesian unit vector and ϵj is a real transverse polarization vector. Let κ(ωj) be the finite-mode coupling coefficient, and let Jαα(t)=Tr⁡[B~α(t)BαρB] for Bα=−d0Eα/γ.

Use the maximal occupation-basis mode operators, identified with their finite-mode symmetric Fock realization as in the thermal-correlator expansion. For this correlator, the field operators are the extensions to D=⋂j=1m(D(aj)∩D(aj†)), with Bα=−γ−1/2∑jPαj[κ(ωj)aj+κ(ωj)∗aj†] on D. Its free conjugate has the same domain. The Gibbs-weighted two-field products are defined on the whole bath space and trace class by that expansion result.

The antinormal contraction is Tr⁡(ajak†ρB)=δjk(1+Nj). Its contribution to the correlator, meaning the part containing annihilation at time t and creation at time zero, is, for real t,

Jαα(t){aa†}=1γ∑j=1mPαj2∣κ(ωj)∣2e−iωjt(1+Nj).

The factor 1 is conventionally called the spontaneous contribution and Nj the stimulated contribution. In the article's continuum notation the corresponding formal expression is ∫d3k∑ε[e^α⋅ε(k)]2∣κ(ω)∣2e−iωt[1+(eβω−1)−1]. The article's equations (S3.9)–(S3.10) display the occupation sum and insert a1a2†=δ12+a2†a1 before its cancellation of partition factors. No continuum limit is established here; absorbing the finite expression's 1/γ requires a consistent redefinition of the coupling or correlator.

Facts & Assumptions

Given: The choice assumptions, positive finite-mode data and physical postulates in the Statement.

[F1]

The regulated bath has finitely many independent positive-frequency modes, and its thermal preparation has the occupation basis, Hamiltonian and partition function stated above. Regularized transverse photon dipole bath model Thermal photon bath and partition function

[F2]

The correlator and dipole coupling use the definition and normalization stated above. Bath correlation matrix and Fourier convention Dimensionless dipole and ULE coupling identification

[F3]

The finite-mode Gibbs products of two ladder operators are trace class; the normal contraction is Tr⁡(ak†ajρB)=δjkNj, and the antinormal contraction is δjk(1+Nj). Finite-mode bosonic Gibbs occupations and moments

[F4]

In the regulated correlator's absolutely convergent occupation expansion, the coefficient of aj at time t is Pαjκ(ωj)e−iωjt/γ, up to the common minus sign of the bath operator, and the coefficient of ak† at time zero is its corresponding conjugate. Photon-number expansion of the diagonal bath correlator

[F5]

The normal occupation sum factors into the selected mode's weighted number sum and the other modes' partition functions, giving Nj after normalization. Thermal contractions and absorption contribution

[F6]

In the finite-mode Fock realization, write ej for the standard orthonormal mode vectors, so aj=a(ej) and aj†=a†(ej). The common invariant finite-particle core Dfin contains every occupation vector. On this core the bosonic identity is ajak†=δjkI+ak†aj, since ⟨ej,ek⟩=δjk. Dimensionless dipole and ULE coupling identification Bosonic and fermionic Fock operators with exact domains

[F7]

Under Countable Choice, a trace-class operator has an absolutely convergent diagonal sum in any supplied Hilbert basis, equal to its trace. Apply the trace theorem to the occupation basis and to each product in [F3]. To match its first-variable-linear convention with the Fock convention, use (u,v)1=⟨v,u⟩2; then (Tu,u)1=⟨u,Tu⟩2. Trace is absolutely convergent and basis independent

[F8]

The thermal-correlator expansion identifies the occupation and symmetric Fock realizations, defines these field extensions on D, proves invariance of that domain under free evolution, and proves that the Gibbs-weighted two-field product is defined on the whole space and trace class. Photon-number expansion of the diagonal bath correlator

Proof

Given: The choice assumptions, positive finite-mode data and physical postulates in the Statement.

Goal: Establish the antinormal contraction, its partition-factor cancellation, and the finite-mode correlator contribution.

1.1F6A1algebra

Each occupation vector lies in Dfin, where [F6] gives ajak†=δjkI+ak†aj. Thus ⟨n∣ajak†∣n⟩=δjk+⟨n∣ak†aj∣n⟩ for every n. This uses only the common-core identity, without asserting equality on unrestricted product domains.

2.1F1F3F7A1step 1.1algebra

By [F1], ρB∣n⟩=pn∣n⟩, where pn=Z−1e−β∑lnlωl, and ∑npn=1. Multiply the diagonal identity in step 1.1 by pn and sum. The two ladder products composed with ρB are trace class by [F3], so [F7] identifies the absolutely convergent diagonal sums with their traces. Consequently Tr⁡(ajak†ρB)=δjk+Tr⁡(ak†ajρB)=δjk(1+Nj), using the normal contraction in [F3].

3.1F1F5step 2.1algebra

Explicitly, put ql=e−βωl. For j=k, the identity part of the occupation sum is Z−1∏l∑nl≥0qlnl=1 by [F1]. The remaining normal part factors and equals Nj by [F5]. For j≠k the Kronecker factor and normal contraction both vanish. This is the finite-mode partition-factor cancellation corresponding to the article's two displayed occupation sums.

4.1F2F4F8step 2.1step 3.1algebra∎

Use the common-domain field realization in [F8]; its trace-class product is the correlator being expanded. Select annihilation at time t and creation at time zero in the finite expansion [F4]. The two common minus signs cancel, and the coefficient multiplying Tr⁡(ajak†ρB) is γ−1PαjPαkκ(ωj)κ(ωk)∗e−iωjt. Step 2.1 leaves only j=k, yielding the displayed finite sum. The real polarization factors give Pαj2, while the coupling product gives ∣κ(ωj)∣2. The calculation uses no continuum interchange or regulator-removal limit.

Source notes

The article's continuum expression and its labels for the two contributions are recorded for attribution. The finite-mode result follows from the stated suppliers and retains the normalization specified by the bath operator; the article citation is not used as its proof.

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