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Photon-number expansion of the diagonal bath correlator

PDF p. 12: Eqs. (S3.4)–(S3.5)

Statement

Assume the Axiom of Choice, Countable Choice and Dependent Choice, and adopt the finite-mode thermal-bath and real-polarization dipole-coupling postulates. Let the finite set of modes be indexed by j=1,…,m, with m≥1, frequencies ωj>0, real transverse polarization vectors ϵj, and β>0. Write Pαj=e^α⋅ϵj and Qj(t)=κ(ωj)∗aj†eiωjt+κ(ωj)aje−iωjt. Here aj and aj† are the mode annihilation and creation operators, e^α is a Cartesian unit vector, and κ contains the selected finite-mode field normalization. For the bath operator Bα=−d0Eα/γ, with γ>0, put Jαα(t)=Tr⁡B[B~α(t)BαρB].

Use the maximal mode operators in the complete occupation-basis realization, identified with the finite-mode symmetric Fock realization by matching occupation vectors. Set D=⋂j=1m(D(aj)∩D(aj†)). In this calculation, Eα and Bα mean the extensions of the initial finite-particle field sums to D, with Bα=−γ−1/2∑jPαjQj(0) there. The free evolution is U(t)∣n⟩=e−itEn∣n⟩, and B~α(t)=U(t)∗BαU(t) has domain U(t)∗D=D. The Gibbs-weighted products in the correlator are defined on the whole bath space and are trace class, as proved below.

Let n=(n1,…,nm)∈N0m, En=∑jnjωj, and Z=∏j(1−e−βωj)−1. Then, for every real t,

Jαα(t)=1γZ∑n⟨n∣∑j,k=1mPαjPαkQj(t)Qk(0)e−βHB∣n⟩=1γZ∑ne−βEn⟨n∣∑j,k=1mPαjPαkQj(t)Qk(0)∣n⟩.

Both series converge absolutely. In particular, with Nj=(eβωj−1)−1,

Jαα(t)=1γ∑j=1mPαj2∣κ(ωj)∣2[Njeiωjt+(Nj+1)e−iωjt].

The article writes the corresponding number-state expansion with continuum mode integrals in equations (S3.4)–(S3.5). Those integrals are formal here: no interchange with an infinite-volume thermal trace or limit of finite-mode expressions is claimed. The explicit factor 1/γ above follows from the stated bath-operator normalization; it may be absorbed only by redefining the coupling coefficients or correlator consistently.

Facts & Assumptions

Given: The mode data, choice assumptions, thermal preparation and coupling postulates in the Statement.

[F1]

For a stationary bath density operator, the bath correlation matrix is defined when every two-time product B~α(t)B~η(s)ρB has a well-defined trace and all resulting entries are invariant under a common time translation. Then Jαη(t−s)=Tr⁡B[B~α(t)B~η(s)ρB]; its diagonal at s=0 is the correlator used here. The channel labels α,η range independently over {x,y,z}. Bath correlation matrix and Fourier convention

[F2]

The finite regulator supplies independent positive-frequency oscillator modes, the complete occupation basis, the maximal shifts aj∣n⟩=nj∣n−ej⟩ (zero for nj=0) and aj†∣n⟩=nj+1∣n+ej⟩, their occupation-weight domains, and diagonal free evolution. Here ej is the unit occupation vector. A continuum thermal preparation and regulator-removal limit require separate specifications. Regularized transverse photon dipole bath model

[F3]

For the finite thermal bath, HB=∑jωjaj†aj and ρB=Z−1e−βHB, with the stated number basis and partition function. Thermal photon bath and partition function

[F4]

In the real-polarization convention, Bα=−d0Eα/γ and the field coefficients are Pαjκ(ωj) for annihilation and their conjugates for creation. Dimensionless dipole and ULE coupling identification

[F5]

In the finite-mode symmetric Fock realization, the occupation vectors form a complete orthonormal basis with the stated diagonal energies and Gibbs weights. For finitely many positive-frequency modes and positive β, every ordered product of two creation or annihilation operators composed with the Gibbs density is defined on the entire bath space and is trace class. Their thermal moments are ⟨aj†ak⟩=δjkNj, ⟨ajak†⟩=δjk(Nj+1), and the moments of two creations or two annihilations vanish. Finite-mode bosonic Gibbs occupations and moments

[F6]

Under Countable Choice, the trace of a trace-class operator equals its absolutely convergent diagonal sum in every supplied Hilbert basis; finite linear combinations remain trace class and their trace is linear. Apply this with the complete occupation basis. To use the trace supplier's first-variable-linear pairing with the Fock second-variable-linear pairing, put (u,v)1=⟨v,u⟩2; then (Tu,u)1=⟨u,Tu⟩2, with unchanged norms and operator domains. Trace is absolutely convergent and basis independent

Proof

Goal: Prove the two number-state expressions, their absolute convergence, and the evaluated finite-mode correlator with the stated field domains.

1.1F2F3F5A1algebra

Match the complete occupation bases in [F2] and [F5]. On finite linear combinations this map preserves the norm and has dense range, so it extends to a unitary identification. The ladder actions agree: the symmetric Fock occupation vectors in [F5] have the raising and lowering actions obtained from their normalized symmetric tensors, and [F2] gives the same coordinate shifts. The maximal domains are exactly the square-summability domains of these weighted coordinates; thus the identification intertwines the maximal mode operators and the diagonal Hamiltonians. Conjugating the first-variable-linear pairing of the tensor realization gives the second-variable-linear Fock convention without changing norms or domains. With ℏ=1, [F2] and [F3] give U(t)∣n⟩=e−itEn∣n⟩. Its modulus-one phases preserve every mode domain. The coordinate shifts therefore give U(t)∗ajU(t)=e−iωjtaj and U(t)∗aj†U(t)=eiωjtaj† on their full maximal domains, including the zero lowering coordinate at nj=0.

2.1F2F4step 1.1algebra

The finite field sum from [F4] extends to the common linear domain D specified in the Statement and agrees with the initial field on finite-particle vectors. By step 1.1, U(t)∗D=D, and conjugation gives B~α(t)=−γ−1/2∑jPαjQj(t) on precisely this domain.

3.1F3F5F6step 2.1algebra

Write L for any one of the finitely many aj,aj†. By [F5], L′LρB is defined on the whole space for every ordered pair L′,L. In particular, ρBψ is in every mode domain and LρBψ is in every mode domain for every bath vector ψ. For every Cartesian channel η and real s, step 2.1 expresses B~η(s) as a finite linear combination of these mode operators on D. Hence B~η(s)ρBψ∈D, and B~α(t)B~η(s)ρB is an actual whole-space operator product for every α,η∈{x,y,z} and t,s∈R. Its finite expansion consists of the trace-class products in [F5], so [F6] makes it trace class. Define its trace to be Cαη(t,s). Substituting [F3] and step 2.1 gives Cαη(t,s)=(γZ)−1Tr⁡B[∑j,kPαjPηkQj(t)Qk(s)e−βHB].

4.1F1F3F5F6step 3.1algebra

Expand each Qj(t)Qk(s) in step 3.1 into its four ladder-operator products. By [F5], the two equal-kind products have zero thermal trace, while the mixed products vanish unless j=k. For j=k, their respective coefficients and moments are ∣κ(ωj)∣2eiωj(t−s)Nj and ∣κ(ωj)∣2e−iωj(t−s)(Nj+1). Trace linearity therefore gives Cαη(t,s)=γ−1∑j=1mPαjPηj∣κ(ωj)∣2[Njeiωj(t−s)+(Nj+1)e−iωj(t−s)] for every channel pair. This depends only on t−s, so Cαη(t+u,s+u)=Cαη(t,s) for every real u. The Gibbs preparation is stationary by [F3], and step 3.1 supplies all nine trace-class products; thus all conditions of [F1] hold for the three-channel matrix. Consequently Jαη(t−s)=Cαη(t,s), including the diagonal at s=0.

5.1F3F5F6step 3.1step 4.1algebra

Each summand in the finite double sum of step 3.1, with η=α and s=0, is trace class by [F5] and e−βHB=ZρB, with 0<Z<∞ from [F3]. Applying [F6] to the supplied occupation basis gives its absolutely convergent diagonal sum; trace linearity permits summing these finitely many series. Also e−βHB∣n⟩=e−βEn∣n⟩ by [F3] and [F5]. These are exactly the two number-state expressions in the Statement. The finite sum of the absolute diagonal sums bounds the absolute sum of the combined series, proving absolute convergence of both expressions without any continuum interchange.

6.1step 3.1step 4.1step 5.1algebra∎

Set η=α and s=0 in step 4.1. The polarization factors become Pαj2, and the surviving terms are ∣κ(ωj)∣2eiωjtNj and ∣κ(ωj)∣2e−iωjt(Nj+1), with the normalization 1/γ from step 3.1. This is the final displayed formula, and step 5.1 supplies both absolutely convergent number-state representations. No continuum limit is used.

Source notes

Equations (S3.4)–(S3.5) of the article use continuum integrations and display the Gibbs operator before replacing it by its occupation-basis eigenvalue. The finite sums above are the regulated counterpart, not a proof that those continuum expressions exist. The article's preceding identification uses Bα=−d0Eα/γ; with the separately stated κ=d0E, that identification yields the displayed 1/γ in the correlator. The conditional calculation makes this normalization explicit without assuming a value of γ.

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